Near-field optical study of active plasmonic sources in the infrared and local spectroscopy of the thermal emission
Arthur Babuty, doctorant - PhD student Crédits : ESPCI ParisTech
We present an apertureless scanning near-field optical microscopy (a-SNOM) analysis of quantum cascade lasers (QCLs) specially designed for the electrical generation of surface plasmonspolaritons (SPPs) in the mid infrared. SPPs are generated either by structuring the top surface of the ridge of the QCL with a metallic gold grating, or by direct coupling at the output facet of the laser with a metallic strip. When this strip is periodically structured, we demonstrate that is possible to give to the mid infrared SPPs confinement properties similar to ones found for visible SPPs on flat metallic surfaces. Shaping the grating end as a tip gives us the possibility to confine the energy of the SPPs on a sub-wavelength hot spot.
We also present the spectroscopy of the near field thermal emission obtained by coupling an a-SNOM – without external illumination - to a Fourier transform infrared spectrometer (FTIR). By studying polar materials which exhibit surface modes called surface phonons-polaritons, we measure their spectrum characterized in the near field by a monochromatic peak. This is the first experimental demonstration of the temporal coherence of the near-field thermal emission. We show that we measure the spectral variations of the local density of photonic states (LDOS) using a theoretical model developed by our collaborators. With this novel instrument, we are thus able to perform infrared spectroscopy with a spatial sub-wavelength resolution.